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Stereoselective Total Syntheses of Tsaokopyranols (–)-E, (–)-L, (+)-M, (+)- Jughopnin J, and (–)-Engelheptanoxide A
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Advisor
이동주
Affiliation
아주대학교 일반대학원
Department
일반대학원 약학과
Publication Year
2022-02
Publisher
The Graduate School, Ajou University
Keyword
(+)-Jughopnin J(+)-Tsaokopyranol M(–)-Engelheptanoxide A(–)-Tsaokopyranol E(–)-Tsaokopyranol LDehydrogenative cycloetherificationDiastereoselectivityNatural Productstrans-2-Alkyl-6-aryl-36-dihydro2H-pyran
Description
학위논문(석사)--아주대학교 일반대학원 :약학과,2022. 2
Alternative Abstract
The stereoselective total syntheses of naturally occurring bioactive 2,6-epoxydiarylheptanoids tsaokopyranols (–)-E, (–)-L, (+)-M, (+)-jughopnin J, and (–)-engelheptanoxide A have been accomplished in 4–6 steps starting from a chiral epoxide utilizing dehydrogenative cycloetherification and epimerization of trans- to cis-2-alkyl-6-aryl-3,6-dihydro-2H-pyran framework as the key steps. The absolute configuration of natural tsaokopyranol L was revised.
Language
eng
URI
https://aurora.ajou.ac.kr/handle/2018.oak/21182
Journal URL
https://dcoll.ajou.ac.kr/dcollection/common/orgView/000000031760
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