Erstwhile, displays using down-converting color changing medium utilized color filters as an essential part of clarifying the trade-off between true colors and transmittance. In this study, we report the development of a novel, smart process for producing thin luminescent films that completely convert colors and enhance light intensity. Highly dense films are prepared by the co-deposition of perovskite quantum dots and metal oxide particles as color conversion layers and scattering agents, respectively. These layers can be directly deposited on blue organic light-emitting diodes using ultrasonic-assisted aerosol deposition (UAD). This method can allow displays using a down-conversion system to streamline the process due to absence of color filters. Using this method, films can be a minimum of 3 µm thick for complete conversion of blue light, a quarter that of inkjet-printed films. We demonstrate 7,353 cd m-2 in green and 411 cd m-2 in red converted emissions with no blue light leakage. Furthermore, the developed technique was shown to be compatible with versatile patterning processes. For example, UAD may be combined with a fine-metal shadow mask to produce a pattern of 30-μm-diameter dots. Even without using a mask, the method still produces a pattern of 13 μm wide lines. This system provides a new approach that may serve as an alternative to inkjet printing.
This study was supported by the National Research Foundation of Korea (NRF) under the Ministry of Science, ICT & Future Planning (Basic Science Research Program (No.2021R1A5A6002853, 2020R1A2C1004943, 2021M3H4A3A01062960, 2020M3A7B4002030, 2020R1A6A1A03048004, 2020R1G1A1102045, 2020R1F1A1073491) and Nano-Material Technology Development Program (No. 2017M3A7B4041696), Republic of Korea. Additionally, this work was supported by a Research Grant from Kwangwoon University in 2021, Korea Institute for Advancement of Technology (KIAT) grant funded by the Korea Government (MOTIE) (P0012451, The Competency Development Program for Industry Specialist) and National Research Facilities & Equipment Center of Korea Basic Science Institute (No. 2019R1A6C1010052).