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Influence of quantum dot concentration on the opto-electronic properties of colloidal quantum-dots LEDs
  • Nguyen, Huu Tuan ;
  • Das, Raja ;
  • Duong, Anh Tuan ;
  • Lee, Soonil
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Publication Year
2020-11-01
Publisher
Elsevier B.V.
Citation
Optical Materials, Vol.109
Keyword
ElectroluminescenceQD concentrationQD EMLQLEDs
Mesh Keyword
CdSe/ZnS quantum dotsCharge recombinationsColloidal quantum dotsExternal quantum efficiencyGreen photoluminescenceLight emitting devicesOperation characteristicOptoelectronic properties
All Science Classification Codes (ASJC)
Electronic, Optical and Magnetic MaterialsComputer Science (all)Atomic and Molecular Physics, and OpticsSpectroscopyPhysical and Theoretical ChemistryOrganic ChemistryInorganic ChemistryElectrical and Electronic Engineering
Abstract
We fabricated and studied the operation characteristics of light emitting devices (LEDs) based on green CdSe/ZnS quantum dots (QDs). A series of devices with different concentrations of QDs in toluene showed typical electroluminescence (EL) peaks that are consistent with green photoluminescence of colloidal QDs emitting layer (EML), but their bandwidth were varied due to the parasitic emission originating from the adjacent organic layers. Upon the increase of the QD concentration, the contribution of the color contamination to emission light from QD-LED (QLED) devices was decreased resulting in the narrowing of EL spectra. On the other hand, the maximum efficiency of QLEDs increased in the lower QD concentration range, while decreased in the higher range. The optimum luminous efficiency of 1.22 cd/A and the external quantum efficiency of 0.43% at standard video brightness (200 cd/m2) was observed from the device with a QD concentration of 6 mg/ml which can be attributed to the enhanced charge recombination in QD EML.
ISSN
0925-3467
Language
eng
URI
https://dspace.ajou.ac.kr/dev/handle/2018.oak/31479
DOI
https://doi.org/10.1016/j.optmat.2020.110251
Fulltext

Type
Article
Funding
We acknowledge financial support from the Vietnam National Foundation for Science and Technology Development (NAFOSTED) under grant number 103.03-2020.09. SL acknowledges support by the “Human Resources Program in Energy Technology” of the Korea Institute of Energy Technology Evaluation and Planning (KETEP), granted financial resource from the Ministry of Trade, Industry & Energy (MOTIE), Republic of Korea (No. 20164030201380), and by the GRRC program of Gyeonggi province [GRRC-AJOU2016B03, Photonics-Medical Convergence Technology Research Center].We acknowledge financial support from the Vietnam National Foundation for Science and Technology Development (NAFOSTED) under grant number 103.03-2020.09 . SL acknowledges support by the “Human Resources Program in Energy Technology” of the Korea Institute of Energy Technology Evaluation and Planning (KETEP) , granted financial resource from the Ministry of Trade, Industry & Energy (MOTIE), Republic of Korea (No. 20164030201380 ), and by the GRRC program of Gyeonggi province [GRRC- AJOU2016B03 , Photonics-Medical Convergence Technology Research Center].
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