We demonstrate subcycle electron pulse generation in a nanogap of graphene when irradiated by a femtosecond laser pulse in the near-infrared region (800 nm). A strong photoinduced emission was produced when the gap area was irradiated by the ultrashort pulse laser. The graphene, which has atomically sharp edges with a large damage threshold, enables us to achieve a strong tunneling regime for the subcycle field emission. The photoinduced signals exhibited an anomalous increase in nonlinear order as a function of incident pulse energy in the presence of static electric field. A dynamical analysis of tunneling electrons based on the semiclassical model, which considers the contribution from the recoil electrons, reproduced our observation successfully. The large field enhancement near the graphene edge enabled us to reach the deep tunneling regime with the extraordinary Keldysh parameter of 0.2 in the near-infrared region, which has not been accessible by conventional metal nanostructures.
This work was supported by the Midcareer Researcher Program (2017R1A2B4009177) and Basic Science Research Program (2015R1D1A1A01061274) through a National Research Foundation grant funded by the Korean government (MSIP) and by Human Resources Program in Energy Technology (20164030201380) of the Korea Institute of Energy Technology Evaluation and Planning (KETEP) grant funded by Korean government (MOTIE).
